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Water-Driven Film Wrinkling with Tunable Modes for Frictional and Optical Applications.
Senjiang Yu1, Bo Yang1, Boyuan Huang2
1Key Laboratory of Novel Materials for Sensor of Zhejiang Province, College of Materials and Environmental Engineering, Hangzhou Dianzi University, Hangzhou 310018, P.R. China.
ACS Applied Materials & Interfaces
|December 13, 2025
Summary
Researchers developed a water-driven method to control wrinkle patterns in metal films on poly(vinyl alcohol) (PVA) substrates. This technique allows for tunable wrinkle modes and arrays, enhancing applications in flexible electronics and optics.
Area of Science:
- Materials Science
- Surface Engineering
- Nanotechnology
Background:
- Wrinkle patterns are common in nature and technology, with applications in flexible electronics, optics, and energy devices.
- Precisely controlling wrinkle formation in real-time and specific regions remains a significant challenge.
Purpose of the Study:
- To investigate water-driven wrinkling in metal films on poly(vinyl alcohol) (PVA) substrates.
- To achieve controllable formation of tunable wrinkle modes and arrays.
Main Methods:
- Sputter-deposition of metal films onto poly(vinyl alcohol) (PVA) substrates.
- Utilizing high humidity and water droplets to reduce PVA modulus and induce wrinkling.
- Investigating wrinkle growth, evolution, morphology, film thickness dependence, and formation mechanisms.
Main Results:
- Water-driven techniques (high humidity, water droplets) enable controllable wrinkle formation by reducing PVA modulus.
- Anisotropic friction observed in striped wrinkles; nearly isotropic friction in herringbone wrinkles.
- Water drop-induced orthogonal wrinkles exhibit unique light diffraction, correlating performance with features.
Conclusions:
- Water-triggered wrinkling provides an efficient method for fabricating tunable wrinkle patterns.
- The study enhances understanding of water-condition-induced wrinkles for practical applications in various fields.

