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Related Experiment Video

Updated: Jan 8, 2026

Quantifying X-Ray Fluorescence Data Using MAPS
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Published on: February 17, 2018

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MapsTorch: automatic differentiation for X-ray fluorescence data analysis.

Xiangyu Yin1, Zichao Di1, Olga Antipova1

  • 1Advanced Photon Source, Argonne National Laboratory, Argonne, IL 60439, USA.

Journal of Synchrotron Radiation
|December 17, 2025
PubMed
Summary

MapsTorch utilizes automatic differentiation to automate X-ray fluorescence (XRF) spectrum fitting, improving elemental analysis efficiency. This open-source tool offers robust parameter optimization, enhancing data analysis for synchrotron experiments.

Keywords:
X-ray fluorescenceautomatic differentiationmachine learningoptimization

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Area of Science:

  • Analytical Chemistry
  • Materials Science
  • Spectroscopy

Background:

  • X-ray fluorescence (XRF) is crucial for elemental analysis.
  • Manual spectrum fitting in XRF is time-consuming, especially for large synchrotron datasets.

Purpose of the Study:

  • Introduce automatic differentiation (AD) to XRF analysis.
  • Develop an open-source package, MapsTorch, for automated XRF data processing.

Main Methods:

  • Transforming analytical XRF models into differentiable computation graphs using AD.
  • Implementing MapsTorch for robust optimization of spectral parameters and elemental intensities.
  • Evaluating MapsTorch against NLopt using historical synchrotron XRF datasets.

Main Results:

  • MapsTorch achieves high-quality XRF spectrum fits.
  • MapsTorch demonstrates superior or comparable fitting quality to NLopt.
  • The tool excels in initial spectrum fitting and elemental intensity refinement.

Conclusions:

  • MapsTorch offers a robust and efficient solution for XRF data analysis.
  • The AD technique streamlines complex spectral fitting processes.
  • MapsTorch facilitates automated, high-throughput analysis for next-generation synchrotron facilities.