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Updated: Jan 8, 2026

Reaction Kinetics and Combustion Dynamics of I4O9 and Aluminum Mixtures
Published on: November 7, 2016
Observation of kinetic mix enhancement in thin-shell OMEGA implosions
B L Reichelt1, M Gatu Johnson1, J H Kunimune1
1Massachusetts Institute of Technology, Cambridge, Massachusetts 02139, USA.
None:
Recent separated reactant experiments for thin-shell (6µm) shock-driven implosions on OMEGA have demonstrated significant mix from a buried deuterated layer of the shell into the hot spot. Time resolved D^{3}He-p reaction history data demonstrate a (50±20)ps shift earlier in peak nuclear emission for separated reactant experiments relative to control, in contrast to past experimental data for thicker, 20µm shells with no laser burn through that show a 75ps delay due to the time required for hydrodynamic instabilities to develop. This contrast suggests that the mix mechanism was not hydrodynamic. Ion kinetic simulations utilizing fall line analyses show much closer agreement with mix yield and temperature than diffusion models, predicting a D^{3}He-p mix yield of 1.7×10^{9} as compared to the experimental value of 9.3(±2.1)×10^{8}. This is three orders of magnitude closer than the fall line analysis from a hydrodynamic simulation with an inline diffusive mix model, which suggests minimal mix and D^{3}He-p yields of 5×10^{5}. This makes kinetic mechanisms the only feasible explanation for the mix seen, demonstrating impact of a non-standard mix mechanism. An analytical model of this kinetic mix mechanism suggests that it can remain significant in situations when the shell expands significantly to low densities, and diffusive models predict negligible mix. Kinetic mix will impact multiple types of high energy density, laser-driven fusion experiments including high-adiabat direct drive cryoexperiments, nuclear cross section experiments, and thin-shell polar direct drive experiments used to tune heat conduction models.
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