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Published on: March 24, 2019
Giant THz Magnetoresistance and Refractive Index Shift in Spin-Textured EuTe2 via Field-Controlled Bandgap
Pengli Hao1,2, Zhuang Ren1,2, Biwen Huang1,2
1High Magnetic Field Laboratory, HFIPS, Chinese Academy of Sciences, Hefei 230031, China.
Abstract:
The realization of terahertz (THz)-frequency magneto effects presents a fundamental challenge and opportunity for ultrafast spintronics. Herein, we demonstrate record-breaking THz giant magnetoresistance (GMR) and anisotropic magnetoresistance (AMR) in EuTe2, a model noncollinear antiferromagnet. Under a 2.5 T magnetic field, the THz GMR exceeds 90%, while the THz AMR reaches an unprecedented 450% at 0.48 THz (2 T) and 5 K, surpassing known MR effects in this frequency regime. Further, THz absorption spectroscopy provides the first direct optical evidence of spin-texture bands via a field-induced bandgap reconstruction from 4.9 to 2.2 meV, linking the THz GMR/AMR to spin-orientation control rather than conventional spin arrangement manipulation. Moreover, a pronounced refractive index shift (Δn ∼ 0.8) results from magnetic field-induced bandgap closure and permeability tuning, a mechanism unlike thermal effects. Our findings promote spin-texture materials as a promising platform for high-frequency spintronics and magneto-optics, while also establishing THz spectroscopy as a transformative tool for probing quantum dynamics.
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