Dynamic Spin Governing Asymmetric Coordination Fields in Trimetallic Single-Atom Catalysts for Optimal Oxygen

Kexin Song1, Binbin Yang1, Wengang An2

  • 1Key Laboratory of Automobile Materials Ministry of Education, School of Materials Science & Engineering, Electron Microscopy Center, Changbaishan Laboratory, International Center of Future Science, Jilin University, Changchun, 130012, P.R. China.

Summary

We developed a "Dynamic Spin Engineering" strategy for tri-metallic single-atom catalysts, enhancing oxygen reduction reaction (ORR) performance and stability. This approach optimizes proton-coupled electron transfer (PCET) by enabling dynamic reconstruction and spin-state transitions in catalysts.

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