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Mobility-induced phase separation in a binary mixture of active Brownian particles.
Daniel Jiménez-Flores1, Álvaro Rodríguez-Rivas2, José Manuel Romero-Enrique1,3
1Departamento de Física Atómica, Molecular y Nuclear, Área de Física Teórica, Facultad de Física, Universidad de Sevilla, Avenida de Reina Mercedes s/n, Sevilla 41012, Spain.
Brownian dynamics simulations reveal that active soft particles in a binary mixture exhibit liquid-like behavior in high-density states, unlike solid-like states in monocomponent systems. This study explores mobility-induced phase separation in two-dimensional systems.
Area of Science:
- Soft Matter Physics
- Statistical Mechanics
- Computational Physics
Background:
- Active matter systems exhibit unique collective behaviors driven by self-propulsion.
- Phase separation is a fundamental phenomenon in condensed matter physics.
- Binary mixtures introduce complexity compared to monocomponent systems.
Purpose of the Study:
- To investigate mobility-induced phase separation in a 2D binary mixture of active soft Brownian particles.
- To characterize the structural and dynamic properties of coexisting phases.
- To compare the behavior of binary mixtures with monocomponent systems.
Main Methods:
- Brownian dynamics simulations were employed.
- Non-additive Weeks-Chandler-Andersen potentials were used to model particle interactions.
- Analysis included radial distribution functions, hexatic order parameter, and mean-square displacement.
Main Results:
- The high-density coexisting state in the binary mixture is spatially disordered and liquid-like.
- Both low- and high-density coexisting states in the binary system show diffusive behavior at long times.
- The monocomponent system's solid-like state also exhibits diffusive behavior due to active topological defects.
Conclusions:
- Active soft particle binary mixtures display distinct phase separation behaviors compared to monocomponent systems.
- The high-density phase in binary mixtures is characterized by liquid-like dynamics.
- Active topological defects play a crucial role in the dynamics of dense active matter systems.
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