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  2. Scalable Carbon Dioxide Capture Using Clay-derived Zeolites Via Atomic Rearrangement.
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Scalable Carbon Dioxide Capture Using Clay-Derived Zeolites via Atomic Rearrangement.

Jinlei Li1, Junyan Li1, Siyuan Fang1

  • 1Department of Materials Science and Engineering, Stanford University, Stanford, California 94305, United States.

Journal of the American Chemical Society
|February 25, 2026

View abstract on PubMed

Summary
This summary is machine-generated.

Researchers developed a scalable method to create a novel carbon capture material from halloysite clay. This new zeolite adsorbent efficiently captures carbon dioxide, offering a promising solution for climate change mitigation.

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Area of Science:

  • Materials Science
  • Chemical Engineering
  • Environmental Science

Background:

  • Effective carbon capture is vital for climate change mitigation and sustainable industry.
  • Developing scalable, cost-effective adsorbents with high CO2 capacity, selectivity, and stability is challenging.

Purpose of the Study:

  • To report the scalable synthesis of Linde Type A zeolite from halloysite clay.
  • To evaluate the CO2 adsorption capacity, selectivity, and stability of the synthesized zeolite.

Main Methods:

  • Scalable synthesis of Linde Type A zeolite via atomic reassembly of halloysite clay.
  • Utilizing mature industrial processes for material transformation.
  • In situ testing for adsorption mechanism and regeneration studies.

Main Results:

  • Achieved high CO2 adsorption capacity (5.0 mmol g⁻¹).
  • Demonstrated outstanding CO2/N2 selectivity (178 for 5% CO2).
  • Exhibited good cyclic stability and robust thermal stability over multiple adsorption-desorption cycles.

Conclusions:

  • The atomic reassembly of halloysite clay provides a scalable strategy for high-performance carbon capture adsorbents.
  • The synthesized zeolite offers a promising solution for gigaton-scale carbon dioxide capture applications.
  • Weakly bound interactions facilitate easy regeneration, enhancing practical applicability.