Error-Resilient Reversal of Quantum Chaotic Dynamics Enabled by Scramblons

The emergence of the arrow of time in quantum many-body systems stems from the inherent tendency of Hamiltonian evolution to scramble quantum information and increase entanglement. While, in principle, one might counteract this temporal directionality by engineering a perfectly inverted Hamiltonian to reverse entanglement growth, such a scenario is fundamentally unstable because even minor imperfections in the backward evolution can be exponentially amplified, a hallmark of quantum many-body chaos. Therefore, successfully reversing quantum many-body dynamics demands a deep understanding of the underlying structure of quantum information scrambling and chaotic dynamics. In this Letter, by using solid-state nuclear magnetic resonance on a macroscopic ensemble of randomly interacting spins, we measure the out-of-time-ordered correlator and validate key predictions of scramblon theory, a universal theoretical framework for information scrambling. Crucially, this theory enables us to isolate and mitigate errors in the out-of-time-ordered correlator caused by imperfections in the backward evolution. As a result, this protocol uncovers the anticipated exponential behavior of quantum many-body chaos and extracts the quantum Lyapunov exponent in a many-body experimental system for the first time. Our results push the fundamental limits of dynamical reversibility of complex quantum systems, with implications for quantum simulation and metrology.