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Preparation of Biopolymer Aerogels Using Green Solvents
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Thermally Processable Adhesive Aerogel Capsules.

Yanchun Han1, Fangshuo Li1, Quan Wang1

  • 1Key Laboratory of Rubber-Plastics, Ministry of Education/Shandong Provincial Key Laboratory of Rubber-plastics, State Key Laboratory of Advanced Optical Polymer and Manufacturing Technology, Qingdao University of Science & Technology, Qingdao, China.

Advanced Materials (Deerfield Beach, Fla.)
|March 2, 2026
PubMed
Summary
This summary is machine-generated.

Researchers developed adhesive aerogel capsules (SAACs) with a core-shell structure. These SAACs offer excellent thermal insulation and adhesion for advanced material applications.

Keywords:
adhesiveaerogel capsulesself‐assemblythermally processable

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Area of Science:

  • Materials Science
  • Nanotechnology

Background:

  • Traditional aerogels possess excellent thermal insulation but suffer from poor adhesion.
  • This limitation hinders their integration into functional systems and broader applications.

Purpose of the Study:

  • To develop novel adhesive aerogel capsules (SAACs) inspired by expanded thermoplastic polyurethane (ETPU) architecture.
  • To overcome the adhesion limitations of conventional aerogels while retaining their desirable properties.

Main Methods:

  • Fabrication of SAACs using a core-shell structure with a chitosan/silica aerogel (CTS/SA) core and a chitosan/carboxylated nitrile rubber (CTS/XNBR) shell.
  • Utilized electrostatically-based self-assembly and freeze-drying for capsule formation.
  • Thermally processed SAACs at mild temperatures (≤ 80°C) for adhesion and assembly.

Main Results:

  • SAACs exhibit a core-shell structure with preserved thermal insulation and enhanced adhesion.
  • Achieved low density, low thermal conductivity (30-39 mW·m-1·K-1), and inherent flame retardancy.
  • Demonstrated thermal processability for adherence to diverse substrates and irregular shapes.

Conclusions:

  • SAACs successfully decouple thermal insulation from adhesion, inspired by ETPU.
  • This novel material combines the benefits of aerogels (insulation, flame retardancy) with the thermal processability of elastomers.
  • SAACs present a versatile platform for on-site thermal management, energy conservation, and fire protection applications.