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Related Concept Videos

Bonding in Metals02:32

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Metallic bonds are formed between two metal atoms. A simplified model to describe metallic bonding has been developed by Paul Drüde called the “Electron Sea Model”.
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The ionic association is the association of oppositely charged ions in an electrolyte solution to form ion pairs. Bjerrum defined ion pairs as two oppositely charged ions whose electrostatic attraction exceeds the thermal energy of the system, typically expressed as 2kT. Electrostatic attraction depends on ionic charge, separation distance, and the dielectric constant of the medium. Thermal energy, represented by kT, reflects the tendency of ions to move independently due to molecular motion.

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Chemical Interaction Customized Metal-Organic Framework Enables Regulated Conductive Network for Selective Superionic

Siting Yu1, Haibin Lu1, Jingqia Weng1

  • 1Guangzhou Key Laboratory of Low-Dimensional Materials and Energy Storage Devices, School of Materials and Energy, Guangdong University of Technology, Guangzhou 510006, China.

Inorganic Chemistry
|March 26, 2026
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Summary
This summary is machine-generated.

Researchers developed new solid-state electrolytes (SSEs) using customized metal-organic frameworks. These advanced SSEs show high ionic conductivity and lithium-ion selectivity, crucial for stable solid-state batteries.

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Nanotechnology

Background:

  • Solid-state electrolytes (SSEs) are critical for safer, high-performance solid-state batteries.
  • Achieving high ionic conductivity, Li+ selectivity, and electrochemical stability simultaneously in processable, air-tolerant SSEs remains a significant challenge.
  • Existing SSEs often compromise on key performance metrics, hindering widespread adoption.

Purpose of the Study:

  • To engineer novel chemical-interaction-customized metal-organic frameworks (CIC-MOF-X) as advanced SSEs.
  • To create a regulated polar network with programmable host-guest interactions for enhanced ion transport.
  • To demonstrate a new strategy for developing selective superionic conductors through coordination-structure engineering.

Main Methods:

  • Nanoconfined polymerization of a polar guest matrix within functionalized MOF nanochannels.
  • Decoration of CIC-MOF-OH with hydroxy groups to tailor host-guest interactions.
  • Characterization of ionic conductivity, Li+ transference number, air stability, and electrochemical performance in Li plating/stripping and full cells.

Main Results:

  • CIC-MOF-OH achieved high ionic conductivity (6.1 × 10-4 S cm-1) and Li+ transference number (0.7 at 30 °C).
  • The material demonstrated excellent air stability, retaining conductivity after 30 days in humid air.
  • Stable Li plating/stripping for 1600 hours and high capacity retention in LiFePO4|Li (96.5%) and NCM811|Li (83% after 150 cycles) full cells were achieved.

Conclusions:

  • Coordination-structure engineering in porous crystals offers a general route to selective superionic conduction.
  • The developed CIC-MOF-OH material addresses key limitations in current SSEs, paving the way for improved solid-state batteries.
  • This approach enables the development of processable, air-tolerant SSEs with a desirable combination of high ionic conductivity and Li+ selectivity.