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Updated: Mar 28, 2026

High Resolution Phonon-assisted Quasi-resonance Fluorescence Spectroscopy
Published on: June 28, 2016
Laser direct writing and Raman Stokes contrast screening of quantum emitter sites in hBN
Tadas Paulauskas1, Julius Janušonis2, Edgaras Markauskas2
1Center for Physical Sciences and Technology, Sauletekio al 3, LT- 10257, Vilnius, Lithuania. tadas.paulauskas@ftmc.lt.
Abstract:
Laser direct writing (LDW) enables the spatially defined creation of room-temperature single-photon emitters (SPEs) in hexagonal boron nitride (hBN). However, the rapid characterization of written sites remains a bottleneck, and the available toolset for efficient screening is limited. Here, we demonstrate a streamlined LDW workflow utilizing single-shot pulses combined with a confocal screening technique that exploits the hBN E2g Stokes line to rapidly localize and map laser-modified regions without relying a priori on defect photoluminescence (PL). This approach enables the direct correlation of site morphology with PL hotspots, revealing that the emergence of single-photon emitters coincides with a threshold regime of minimal lattice modification. Micro-Raman spectral mapping further uncovers localized compressive strain surrounding these emission sites. We classify the generated defects into two families: narrowband "red" emitters (650-750 nm) with weak phonon sidebands (PSB), and 600-650 nm emitters with stronger vibronic coupling, both exhibiting linear polarization and high single-photon purity. These results establish a practical protocol for rapid prototyping, offering a valuable addition to the characterization toolkit for scalable quantum nanophotonics.
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