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Shengliang Zhang1,2, Junhua Zhou1, Zekun Huang1

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This study introduces a flexible multicolor dynamic radiative modulator (MDRM) for intelligent building thermal regulation. The novel device enhances energy efficiency by dynamically tuning thermal radiation, offering a sustainable solution for buildings.

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Area of Science:

  • Materials Science
  • Energy Science
  • Nanotechnology

Background:

  • Dynamic radiative modulators offer potential for building energy savings by tuning mid-infrared emissivity.
  • Current limitations include poor color tunability, slow switching, and short device lifespans, hindering practical application.

Purpose of the Study:

  • To design and demonstrate a flexible multicolor dynamic radiative modulator (MDRM) for intelligent thermal regulation in buildings.
  • To overcome the limitations of existing technologies by improving tunability, switching speed, and cycling life.

Main Methods:

  • Fabrication of a flexible MDRM using a polyaniline nanorod cathode and a Zn2+-based quasi-solid gel electrolyte.
  • Characterization of the device's electrochromic performance, including multiband modulation, switching speed, and cycling stability.
  • Evaluation of the temperature regulation capability of the MDRM.

Main Results:

  • The flexible MDRM demonstrated high multiband modulation (visible to MIR) with ΔR = 0.32 and Δε = 0.34.
  • The device exhibited fast switching speeds and good cycling stability, retaining 75.6% capacity after 2000 cycles.
  • The MDRM achieved a significant temperature regulation of 8.8 °C.

Conclusions:

  • The developed flexible MDRM offers multicolor tunability and dynamic thermal radiation modulation for building envelopes.
  • The device shows great potential for energy-efficient building thermal management, contributing to sustainability goals.
  • This work presents a viable strategy for creating advanced radiative modulators for energy savings and carbon neutrality.