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Multiscale Design Strategies for Fast-Charging Graphite Anodes in Lithium-Ion Batteries.

Weijie Hu1,2,3, Yanmi Pan1,3, Mingjian Zhong1,3

  • 1School of Chemistry, Guangdong University of Petrochemical Technology, Maoming, Guangdong, China.

Small (Weinheim an Der Bergstrasse, Germany)
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PubMed
Summary
This summary is machine-generated.

Developing fast-charging lithium-ion batteries requires overcoming graphite anode limitations. This review outlines multiscale challenges and design strategies for improved performance and stability in next-generation batteries.

Keywords:
fast‐charging performancegraphite anodeinterface engineeringlithium‐ion batteriesmultiscale design

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Energy Storage

Background:

  • Graphite anodes limit fast-charging lithium-ion batteries due to sluggish kinetics and interfacial instability.
  • Challenges span atomic-level desolvation to macroscopic ion transport limitations.

Purpose of the Study:

  • To systematically analyze multiscale challenges restricting graphite anode fast-charging performance.
  • To establish a comprehensive design framework for optimizing graphite anodes.
  • To examine dynamic failure mechanisms and industrialization potential.

Main Methods:

  • Review and analysis of multiscale challenges in graphite anodes.
  • Framework development for interfacial engineering, bulk structure modulation, and electrode architecture.
  • Examination of failure mechanisms using in-situ diagnostic techniques.

Main Results:

  • Identified key strategies: artificial SEI, electrolyte tuning, particle morphology control, and gradient electrodes.
  • Critically examined dynamic failure mechanisms like lithium plating and SEI degradation.
  • Assessed industrialization potential and cost-effectiveness of proposed approaches.

Conclusions:

  • Integrated insights and forward-looking perspectives for scalable, high-performance graphite anodes.
  • Development of next-generation fast-charging lithium-ion batteries is feasible through targeted design strategies.
  • Overcoming graphite anode limitations is crucial for advancing electric vehicles and consumer electronics.