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MXene nanosheets create conductive composites by stabilizing emulsions. This study links emulsion microstructure to viscoelastic and electrical properties, revealing MXene networks enhance conductivity.

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Area of Science:

  • Materials Science
  • Colloid and Interface Science

Background:

  • MXene nanosheets are effective stabilizers for emulsion-templated conductive composites.
  • MXene networks at droplet interfaces lead to materials with low percolation thresholds and strong electrical conductivity.

Purpose of the Study:

  • To investigate the relationship between microstructure, viscoelasticity, and functional properties of MXene-stabilized emulsions.
  • To understand how interfacial networks and droplet interactions influence bulk conductivity.

Main Methods:

  • Interfacial and bulk rheology
  • Broadband dielectric spectroscopy
  • Microscopy
  • Rheo-dielectric and rheo-optical characterizations

Main Results:

  • A direct correlation was found between the rheological behavior of the MXene interfacial network and its electrical conductivity.
  • Bulk conductivity in MXene-based Pickering emulsions is influenced by both the interfacial network and droplet-droplet interactions.
  • Emulsion microstructure significantly impacts electrical conductivity and rheological properties under shear and during recovery.

Conclusions:

  • MXene-stabilized emulsions offer a versatile platform for creating conductive composites.
  • Understanding the interplay between microstructure and interfacial properties is crucial for tailoring material performance.
  • This work provides insights into designing advanced functional materials using MXene-based Pickering emulsions.