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Screening of Coatings for an All-Solid-State Battery Using In Situ Transmission Electron Microscopy
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Published on: January 20, 2023

Perspective on Material Design and Interface Engineering toward Low-Stack-Pressure All-Solid-State Lithium Batteries.

Shenghan Gao1,2, Wen-Peng Wang1,2, Li-Jun Wan1,2

  • 1CAS Key Laboratory of Molecular Nanostructure and Nanotechnology, Beijing National Laboratory For Molecular Sciences (BNLMS), Institute of Chemistry, Chinese Academy of Sciences (CAS), Beijing, P. R. China.

Advanced Materials (Deerfield Beach, Fla.)
|May 11, 2026
PubMed
Summary
This summary is machine-generated.

All-solid-state lithium batteries (ASSLBs) need high pressure for good performance. This review explores solutions for low-pressure ASSLBs, focusing on materials and interfaces for better energy storage.

Keywords:
all‐solid‐state batterieselectrode materialsinterfaceslithium batteriessolid electrolytes

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Energy Storage

Background:

  • All-solid-state lithium batteries (ASSLBs) offer high energy density and safety.
  • Poor solid-solid interfacial contact limits ASSLB cyclability and requires high stack pressure.
  • Current limitations hinder the commercialization of ASSLBs.

Purpose of the Study:

  • To provide a fundamental understanding of stack pressure's role in ASSLBs.
  • To analyze challenges in achieving optimal performance under low-stack-pressure conditions.
  • To summarize recent advances in reducing high-stack-pressure demands.

Main Methods:

  • Review of existing literature on ASSLB stack pressure.
  • Analysis of material design (solid electrolyte/active electrode) for low-pressure operation.
  • Examination of interface engineering strategies.

Main Results:

  • High stack pressure is often necessary due to interfacial resistance.
  • Material-centered solutions and interface engineering are key to reducing pressure requirements.
  • Progress has been made in designing components for low-pressure ASSLBs.

Conclusions:

  • Achieving low-stack-pressure ASSLBs is crucial for commercialization.
  • Future breakthroughs require continued focus on material design and interface engineering.
  • Material-centered solutions hold promise for advancing battery technology.