High-Performance Terahertz Detection via Quasi-2D Perovskite/Weyl Semimetal Heterojunction

Terahertz radiation exhibits significant potential for communications, imaging, and spectroscopy. However, the development of efficient and low-cost THz detectors remains challenging due to limitations such as insufficient sensitivity, slow response speed, and poor room temperature stability. This work presents an innovative quasi-2D perovskite/Weyl semimetal (Co₃Sn₂S₂) heterojunction THz detector that combines complementary material properties via band engineering. The device achieves a remarkable responsivity of 374.15 A/W, a specific detectivity of 6.27 × 10¹¹ cm·Hz^1/2·W^-1, and a noise-equivalent power of 0.29 pW·Hz^-1/2 at 0.1 THz. This performance stems from the strong THz absorption of the perovskite layer combined with the high carrier mobility and topological surface states of the Co₃Sn₂S₂, which collectively enable ultrafast carrier extraction and suppressed interfacial recombination. This heterojunction design offers a novel strategy for high-performance terahertz detection and facilitates its integration into next-generation portable, integrated devices.