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Zinc-Sponge Battery Electrodes that Suppress Dendrites

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Dry-Crafted Charge-Conductive ZrO₂ _- _x Cathode Shell Coating for High-Performance Sulfide-Based Solid-State

Yoo Jung Choi¹, Hongjun Chang², Sungbin Jang³

¹Department of Chemical and Biological Engineering, Sookmyung Women's University, Seoul, Republic of Korea.

Small (Weinheim an Der Bergstrasse, Germany)

|May 20, 2026

Summary

This summary is machine-generated.

Researchers developed a novel ZrO2-x coating for lithium-ion battery cathodes, significantly improving the stability of all-solid-state batteries (ASSBs) by preventing interfacial degradation and enhancing performance.

Keywords:

Li6PS5Cl all‐solid‐state batteries mechanofusion oxygen‐deficient ZrO2−x single‐crystalline cathode

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Screening of Coatings for an All-Solid-State Battery Using In Situ Transmission Electron Microscopy

Screening of Coatings for an All-Solid-State Battery Using In Situ Transmission Electron Microscopy

Published on: January 20, 2023

Area of Science:

Materials Science
Electrochemistry
Battery Technology

Background:

All-solid-state batteries (ASSBs) promise higher energy density and safety.
Interfacial instability between sulfide electrolytes and Ni-rich cathodes hinders ASSB cycling stability.

Purpose of the Study:

To mitigate interfacial side reactions in sulfide-based ASSBs.
To enhance the cycling stability of LiNi0.8Mn0.1Co0.1O2 (NMC) cathodes.

Main Methods:

Applied a charge-conductive, black ZrO2-x (BZOx) shell coating to NMC cathodes.
Utilized a solvent-free, dry-processed mechanofusion method for coating.
Compared BZOx-coated NMC with pristine NMC and white ZrO2-coated NMC.

Main Results:

BZOx coating suppressed electrolyte decomposition and interfacial degradation.
Minimized charge-transfer resistance and enhanced Li ion/electron transport.
BZOx-coated NMC showed improved cycling stability, higher coulombic efficiency, and reduced voltage hysteresis.

Conclusions:

Dry-processed BZOx coating effectively stabilizes the cathode-electrolyte interface in ASSBs.
This strategy enhances long-term operation stability for sulfide-based ASSBs.
Charge-conductive ZrO2-x offers a viable pathway for advanced ASSB development.