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Developing Photosensitizer-Cobaloxime Hybrids for Solar-Driven H2 Production in Aqueous Aerobic Conditions
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Lewis-Base Coordination Enables Highly Dispersed Pt Cocatalyst on Pyrene-Based MOFs for Enhanced Photocatalytic

Shuaiqi Guo1, Haibing Meng1, Gang Yu1

  • 1College of Chemistry and Chemical Engineering, Taiyuan University of Technology, Taiyuan, People's Republic of China.

Angewandte Chemie (International Ed. in English)
|May 28, 2026
PubMed
Summary

We engineered platinum (Pt) cocatalyst coordination on metal-organic frameworks (MOFs) using Lewis-base groups. This optimized electronic metal-support interactions (EMSI), significantly boosting photocatalytic hydrogen evolution activity and stability.

Keywords:
Lewis‐base functionalizationcharge separationcoordination structureelectronic metal‐support interactionsmetal‐organic frameworks

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