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Related Experiment Video

Updated: Jun 17, 2026

A Fabrication and Measurement Method for a Flexible Ferroelectric Element Based on Van Der Waals Heteroepitaxy
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A Fabrication and Measurement Method for a Flexible Ferroelectric Element Based on Van Der Waals Heteroepitaxy

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Decoupling Surface Rigidity from Bulk Compliance in Elastomeric Electrolytes via Surface-Architected MXene Interphase

Zhisong Geng1, Yun Xing1, Chenxi Cao1

  • 1MOE Key Laboratory of Resources and Environmental System Optimization, College of Environmental Science and Engineering, North China Electric Power University, Beijing 102206, P. R. China.

Journal of the American Chemical Society
|June 16, 2026
PubMed
Summary

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Surface-engineered elastomeric electrolytes with MXene interphases prevent lithium dendrites, enhancing battery safety and longevity. This breakthrough enables stable, high-energy-density flexible lithium-metal batteries.

Area of Science:

  • Materials Science
  • Electrochemistry
  • Polymer Science

Background:

  • Elastomeric electrolytes offer good interfacial contact but struggle with mechanical strength to prevent lithium dendrites.
  • Lithium dendrites are a major safety concern and performance limitation in lithium-metal batteries.

Purpose of the Study:

  • To engineer a robust interphase for elastomeric electrolytes to overcome mechanical limitations.
  • To improve the ionic conductivity and lithium-ion transport within the electrolyte.
  • To demonstrate stable cycling performance in flexible lithium-metal batteries.

Main Methods:

  • Surface-architected MXene interphase engineering on a hydrogenated nitrile butadiene rubber (HNBR) matrix.
  • Utilizing a high-modulus MXene surface layer for mechanical suppression of dendrites.

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Last Updated: Jun 17, 2026

A Fabrication and Measurement Method for a Flexible Ferroelectric Element Based on Van Der Waals Heteroepitaxy
10:40

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Published on: April 8, 2018

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  • Incorporating a lithiophilic, oriented MXene network to enhance ion flux.

    • Main Results:

    • Achieved an ionic conductivity of 8.05 × 10-4 S cm-1 with enhanced Li+ transport.
    • Demonstrated dendrite-free cycling exceeding 7000 hours.
    • Enabled stable full-cell operation with high-loading LiFePO4 and high-voltage NCM622.

    Conclusions:

    • Surface-bulk mechanical decoupling is a viable strategy for developing high-energy-density, flexible lithium-metal batteries.
    • MXene interphase engineering significantly enhances the mechanical and electrochemical performance of elastomeric electrolytes.
    • The developed strategy offers a generalizable design principle for advanced battery technologies.