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Experimental Study of the Relationship Between Particle Size and Methane Sorption Capacity in Shale
Published on: August 2, 2018
Two decades of methane budgets at the sub-national scale in China
Pengfei Zhao1, Zhen Zhang2, Guanghui Huang3
1College of Earth and Environmental Sciences, Lanzhou University, Lanzhou 730000, China; State Key Laboratory of Tibetan Plateau Earth System, Environment and Resources, Institute of Tibetan Plateau Research, Chinese Academy of Sciences, Beijing 100101, China; National Tibetan Plateau Data Center, Institute of Tibetan Plateau Research, Chinese Academy of Sciences, Beijing 100101, China.
Abstract:
Accurate accounting of regional methane (CH4) emissions and removals is essential for tracking national climate mitigation progress and assessing potential carbon-climate feedbacks. China is the world's largest CH4 emitter, yet comprehensive sub-national estimates remain limited, constraining the development of effective mitigation strategies. This study analyzes CH4 emissions across China from 2000 to 2019 using atmospheric inversion ensembles (top-down approach, TD) and process-based model estimates (bottom-up approach, BU). The datasets for both approaches were contributed by international research teams coordinated through the Global Carbon Project. The spatial distribution of various CH4 fluxes exhibits high spatial heterogeneity. Approximately 60% of national CH4 emissions come from three of the nine sub-national regions (North China, Southeast China, and Southwest China), which together account for <30% of China's land area. These emissions are dominated by the energy and agricultural sectors. Natural sources contribute 9%-16% of the total CH4 budget, but they have the largest relative uncertainties, reaching approximately 150%-170% of their estimated magnitudes. This high uncertainty partly reflects the limited number of studies on natural CH4 sources. The increase in anthropogenic emissions is the primary driver of the changes between the two decades, with increases of 10.4 [2.7-16.9] Tg CH4 a-1 (BU) and 6.1 [-2.6-10.7] Tg CH4 a-1 (TD). The largest increases occur in North China, Southwest China, Southeast China, and Northeast China. This study highlights the need for improved regional monitoring of CH4 emissions and sinks in China to support integrated and spatially targeted mitigation strategies.

