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Regulation Roles of p-Block Elements in Lithium Layered Oxide Cathodes: Recent Progress and Perspectives.

Qian Zhang1, Yuanyuan Zhang1, Xue Ke1

  • 1Institute of Science and Technology for New Energy, Xi'an Technological University, Xi'an, Shanxi, China.

Advanced Materials (Deerfield Beach, Fla.)
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PubMed
Summary

Substituting p-block elements into layered oxides (LixTMyO2) enhances lithium-ion battery (LIB) performance by stabilizing structure and improving kinetics. This review clarifies substitution effects for advanced LIB cathode design.

Keywords:
dopinglayered oxide cathodeslithium‐ion batteriesp‐block elementsstructure regulation

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Chemical Engineering

Background:

  • Layered oxides (LixTMyO2) are crucial for lithium-ion batteries (LIBs) but suffer from structural instability and interface reactions.
  • Substitution with p-block elements offers a promising strategy to overcome these limitations in LIB cathodes.
  • A systematic review is needed to understand the structure-performance relationships governed by p-block element substitution.

Purpose of the Study:

  • To systematically review the role of p-block element substitution in LixTMyO2 cathodes.
  • To elucidate the mechanisms by which p-block elements enhance electrochemical performance.
  • To provide design guidelines for high-performance LIB cathodes.

Main Methods:

  • Literature review of studies on p-block element substitution in LixTMyO2 cathodes.
  • Analysis of structural evolution, diffusion kinetics, and interface reactions.
  • Categorization of substitution effects based on p-block element groups.

Main Results:

  • P-block element substitution effectively mitigates structural degradation and parasitic reactions in LixTMyO2 cathodes.
  • Specific p-block elements demonstrate unique benefits for improving ionic/electronic conductivity and interfacial stability.
  • The review provides a comprehensive overview of substitution strategies and their impact on LIB performance.

Conclusions:

  • P-block element substitution is a key strategy for developing advanced LIB cathodes.
  • Understanding the interplay between substitution, structure, and performance is critical for rational material design.
  • Future research should focus on optimizing substitution patterns and exploring novel p-block elements for enhanced LIBs.