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A battery is a galvanic cell that is used as a source of electrical power for specific applications. Modern batteries exist in a multitude of forms to accommodate various applications, from tiny button batteries such as those that power wristwatches to the very large batteries used to supply backup energy to municipal power grids. Some batteries are designed for single-use applications and cannot be recharged (primary cells), while others are based on conveniently reversible cell reactions that...
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Reliable and Reusable All-Solid-State Contact-Type Pre-Lithiation Platform for High-Performance All-Solid-State

Yunho Lee1,2, Yongjun Kwon3, Juhyeong Noh1,2

  • 1Smart Materials Research Section, Electronics and Telecommunications Research Institute (ETRI), Daejeon, Republic of Korea.

Advanced Materials (Deerfield Beach, Fla.)
|July 8, 2026
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Summary

Researchers developed a reusable pre-lithiation platform for all-solid-state batteries. This method improves initial cycling efficiency and overall performance, enabling higher energy density in solid-state batteries.

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Energy Storage

Background:

  • All-solid-state batteries offer high energy density and safety.
  • Lithium loss and interfacial issues limit their performance.
  • Anode irreversibility and electrolyte instability cause energy density reduction.

Purpose of the Study:

  • To introduce a novel contact-type pre-lithiation platform for all-solid-state batteries.
  • To address lithium loss and interfacial phenomena in solid-state systems.
  • To enhance the electrochemical performance and energy density of all-solid-state batteries.

Main Methods:

  • Developed a reusable contact-type pre-lithiation platform using solid electrolytes and electron-conductive agents.
  • Utilized balanced ionic and electronic transport for uniform electrode pre-lithiation via physical contact.
  • Controlled pre-lithiation with contact time and temperature under low stack pressure (8 MPa).

Main Results:

  • Achieved uniform pre-lithiation of all-solid-state electrodes through reversible physical contact.
  • Low stack pressure suppressed resistive decomposition product formation at the interface.
  • Precisely pre-lithiated anodes optimized interfacial characteristics, enhancing initial Coulombic efficiency and cycling performance.

Conclusions:

  • The developed platform enables effective pre-lithiation for all-solid-state batteries.
  • Optimized interfacial characteristics lead to significantly improved battery performance.
  • This approach contributes to realizing high-performance all-solid-state batteries with high energy density.