Editable Hydrogen Bond Network Within the Electric Double Layer for CO2 Reduction

Jiahao Yang1,2, Shiju Yu3, Jiapeng Jiao4

  • 1Beijing National Laboratory for Molecular Sciences, CAS Laboratory of Colloid and Interface and Thermodynamics, CAS Research/Education Centre for Excellence in Molecular Sciences, Centre for Carbon Neutral Chemistry, Institute of Chemistry, Chinese Academy of Sciences, Beijing, China.

Summary

Altering the water hydrogen bond network (HBN) rigidity at electrified interfaces impacts CO2 electroreduction. Moderate HBN rigidity optimizes C2+ production, achieving 90.9% Faradaic efficiency with a copper electrode.

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