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Related Experiment Video

Updated: Jul 10, 2026

Characterization of Electrode Materials for Lithium Ion and Sodium Ion Batteries Using Synchrotron Radiation Techniques
10:03

Characterization of Electrode Materials for Lithium Ion and Sodium Ion Batteries Using Synchrotron Radiation Techniques

Published on: November 11, 2013

A lithium-ion conductive polymeric coating enables high-performance silicon anodes.

Kang Lu1, Kevin Velasquez Carballo1, Taohedul Islam1

  • 1Department of Mechanical Engineering, University of Arkansas, Fayetteville, AR 72701, USA. xbmeng@uark.edu.

Dalton Transactions (Cambridge, England : 2003)
|July 8, 2026
PubMed
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Researchers developed a novel polymer coating for silicon anodes in lithium-ion batteries. This coating enhances stability and capacity, addressing key challenges for electric vehicle batteries.

Area of Science:

  • Materials Science
  • Electrochemistry
  • Battery Technology

Background:

  • Lithium-ion batteries (LIBs) are dominant in portable electronics but face limitations for transportation applications.
  • Silicon (Si) anodes offer high capacity and cost-effectiveness but suffer from volume changes during cycling.

Purpose of the Study:

  • To address the volume change issue in silicon anodes for LIBs.
  • To develop a protective coating for silicon electrodes using molecular layer deposition (MLD).

Main Methods:

  • Conformal coating of silicon electrodes with a lithium-containing cross-linked polymer (LiGL).
  • Deposition via molecular layer deposition (MLD) using lithium tert-butoxide (LTB) and glycerol (GL) precursors.
  • Electrochemical cycling and characterization of coated silicon electrodes.

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Screening of Coatings for an All-Solid-State Battery Using In Situ Transmission Electron Microscopy
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Screening of Coatings for an All-Solid-State Battery Using In Situ Transmission Electron Microscopy

Published on: January 20, 2023

Focused Ion Beam Fabrication of LiPON-based Solid-state Lithium-ion Nanobatteries for In Situ Testing
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Focused Ion Beam Fabrication of LiPON-based Solid-state Lithium-ion Nanobatteries for In Situ Testing

Published on: March 7, 2018

Related Experiment Videos

Last Updated: Jul 10, 2026

Characterization of Electrode Materials for Lithium Ion and Sodium Ion Batteries Using Synchrotron Radiation Techniques
10:03

Characterization of Electrode Materials for Lithium Ion and Sodium Ion Batteries Using Synchrotron Radiation Techniques

Published on: November 11, 2013

Screening of Coatings for an All-Solid-State Battery Using In Situ Transmission Electron Microscopy
07:20

Screening of Coatings for an All-Solid-State Battery Using In Situ Transmission Electron Microscopy

Published on: January 20, 2023

Focused Ion Beam Fabrication of LiPON-based Solid-state Lithium-ion Nanobatteries for In Situ Testing
10:58

Focused Ion Beam Fabrication of LiPON-based Solid-state Lithium-ion Nanobatteries for In Situ Testing

Published on: March 7, 2018

Main Results:

  • LiGL-coated Si electrodes achieved a reversible capacity of ~838 mAh g⁻¹ after 100 cycles at 0.1C.
  • The LiGL coating acted as an ion-conductive artificial solid electrolyte interphase (SEI).
  • The coating protected Si electrodes from undesirable reactions and accommodated volume changes, improving mechanical integrity.

Conclusions:

  • A novel MLD-based polymer coating effectively enhances the performance and stability of silicon anodes.
  • This approach offers a promising solution for developing next-generation batteries for transportation.
  • MLD presents a versatile technique for addressing challenges in advanced battery materials.