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Applications of Dynamic Polymers in Next-Generation High-Performance Lithium-Based Batteries.

Chang Yan1,2, Leiyu Chen1,2, Wangmao Tian1,2

  • 1Beijing National Laboratory For Molecular Sciences (BNLMS), Laboratory of Polymer Physics and Chemistry, Institute of Chemistry, Chinese Academy of Sciences, Beijing, China.

Advanced Materials (Deerfield Beach, Fla.)
|July 9, 2026
PubMed
Summary
This summary is machine-generated.

Dynamic polymers offer self-healing and recyclable solutions for lithium-based batteries (LBBs). Their adaptable networks improve interface stability, suppress dendrites, and enable sustainable battery design.

Keywords:
dynamic polymerslithium‐based batteriesrecyclabilityself‐healingsustainable energy storage

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Polymer Chemistry

Background:

  • Dynamic polymers possess reversible networks crucial for advanced material functionalities.
  • Lithium-based batteries (LBBs) face challenges like unstable interfaces, mechanical-ionic conductivity trade-offs, and sustainability issues.
  • Dynamic polymers present a promising solution for next-generation LBBs.

Purpose of the Study:

  • To review recent advancements in dynamic polymers for LBB applications.
  • To explore design strategies, mechanisms, and performance of dynamic polymers in electrolytes, interfaces, and binders.
  • To highlight the role of dynamic polymer chemistry in enhancing battery performance and sustainability.

Main Methods:

  • Literature review of dynamic polymer applications in LBBs.
  • Analysis of dynamic bond chemistry (e.g., hydrogen, disulfide, boronate ester, imine bonds) and network dynamics.
  • Evaluation of electrochemical performance and interfacial properties.

Main Results:

  • Dynamic polymers enhance interfacial stability and suppress lithium dendrite growth.
  • They accommodate electrode volume changes and improve the mechanical robustness-ionic conductivity balance.
  • Applications include polymer electrolytes, interface engineering, and binder development for LBBs.
  • Closed-loop recycling of battery components is enabled by dynamic polymer recyclability.

Conclusions:

  • Dynamic polymers are key to developing high-energy-density, long-cycle-life, safe, and sustainable LBBs.
  • Further research into rational design of smart and eco-friendly dynamic polymer battery materials is needed.
  • Addressing current challenges will accelerate the realization of advanced LBB technologies.