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Related Experiment Video

Updated: Jul 12, 2026

Focused Ion Beam Fabrication of LiPON-based Solid-state Lithium-ion Nanobatteries for In Situ Testing
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Anion-Solvent Dual-Sieving Effect Revolutionizes Li Deposition Kinetics for Garnet-Based Solid-State Lithium

Jiaxin Wu1,2, Zichang You1,2, Huayan Huang1,2

  • 1The State Key Lab of High Performance Ceramics and Superfine Microstructure, Shanghai Institute of Ceramics, Chinese Academy of Sciences, Shanghai, P.R. China.

Small (Weinheim an Der Bergstrasse, Germany)
|July 9, 2026
PubMed
Summary

A new composite interlayer (BN-ASDSI) enhances solid-state battery performance by stabilizing the lithium metal interface and improving ion transport, enabling higher critical current densities and longer cycle life for next-generation energy storage.

Keywords:
BN‐nanosheetsLi metal anodesanion‐solvent dual‐sieving effectinterface engineeringoxide‐based solid‐state batteries

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Solid-state Graft Copolymer Electrolytes for Lithium Battery Applications
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Solid-state Graft Copolymer Electrolytes for Lithium Battery Applications

Published on: August 12, 2013

Area of Science:

  • Materials Science
  • Electrochemistry
  • Energy Storage

Background:

  • Solid-state batteries (SSBs) offer high theoretical energy density but face challenges with Li/solid-state electrolyte interfaces.
  • Interfacial issues include poor contact, lithium dendrites, side reactions, and polarization, hindering practical application.
  • Existing solutions often fail to address multiple interfacial problems simultaneously.

Purpose of the Study:

  • To develop a multifunctional composite interlayer (BN-ASDSI) to overcome Li/solid-state electrolyte interfacial limitations in SSBs.
  • To improve lithium-ion transport, suppress dendrite formation, and enhance interfacial stability.
  • To demonstrate the practical viability of BN-ASDSI for high-performance SSBs.

Main Methods:

  • Fabrication of a composite interlayer (BN-ASDSI) using a polymer scaffold, sultone-based electrolyte, and boron nitride (BN).
  • Investigation of interfacial mechanisms, including anion anchoring and solvent-repelling properties.
  • Electrochemical testing of symmetric cells and full cells (LiFePO4 and LiNi0.83Co0.12Mn0.05O2 cathodes) to evaluate performance metrics.

Main Results:

  • BN-ASDSI demonstrated an anion-anchoring effect, promoting Li+ transport and forming a LiF-rich interface for stable Li metal.
  • Symmetric cells achieved an ultrahigh critical current density of 8.8 mA cm-2.
  • LiFePO4 SSBs operated for 1500 cycles at 6C with >92% capacity retention; high-loading NMC SSBs achieved 3.2 mAh cm-2 at 1C with 93% retention after 80 cycles.

Conclusions:

  • The BN-ASDSI interlayer effectively addresses critical interfacial issues in solid-state batteries.
  • This composite interlayer significantly enhances ionic conductivity, interfacial stability, and overall battery performance.
  • BN-ASDSI shows great promise for the development of practical, high-energy-density solid-state batteries.