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Related Concept Videos

Ionic Crystal Structures02:42

Ionic Crystal Structures

Ionic crystals consist of two or more different kinds of ions that usually have different sizes. The packing of these ions into a crystal structure is more complex than the packing of metal atoms that are the same size.
Most monatomic ions behave as charged spheres, and their attraction for ions of opposite charge is the same in every direction. Consequently, stable structures for ionic compounds result (1) when ions of one charge are surrounded by as many ions as possible of the opposite...
Ionic Bonding and Electron Transfer02:48

Ionic Bonding and Electron Transfer

Ions are atoms or molecules bearing an electrical charge. A cation (a positive ion) forms when a neutral atom loses one or more electrons from its valence shell, and an anion (a negative ion) forms when a neutral atom gains one or more electrons in its valence shell. Compounds composed of ions are called ionic compounds (or salts), and their constituent ions are held together by ionic bonds: electrostatic forces of attraction between oppositely charged cations and anions.

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Updated: Jul 14, 2026

Screening of Coatings for an All-Solid-State Battery Using In Situ Transmission Electron Microscopy
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Modulating Local Structure of Amorphous Oxyhalide to Achieve High-Rate and Ultra-Stable All-Solid-State Lithium

Zecheng Fang1, Tao Liu1, Xinglong Jiang1

  • 1Center of Materials Science and Optoelectronics Engineering, College of Materials Science and Optoelectronic Technology, University of Chinese Academy of Sciences, Beijing, P. R. China.

Advanced Materials (Deerfield Beach, Fla.)
|July 13, 2026
PubMed
Summary

This study developed a novel amorphous solid electrolyte (LTOC-M) for halides-based all-solid-state lithium batteries (ASSLBs). The new electrolyte significantly improves ionic conductivity, rate capability, and cycling stability, enabling better low-temperature performance for ASSLBs.

Keywords:
all‐solid‐state batteriesamorphoushalide solid electrolyteslocal structureoxyhalides

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Synthesis of Ionic Liquid Based Electrolytes, Assembly of Li-ion Batteries, and Measurements of Performance at High Temperature
11:04

Synthesis of Ionic Liquid Based Electrolytes, Assembly of Li-ion Batteries, and Measurements of Performance at High Temperature

Published on: December 20, 2016

Area of Science:

  • Materials Science
  • Electrochemistry
  • Solid-State Chemistry

Background:

  • Halides-based all-solid-state lithium batteries (ASSLBs) offer advantages like wide electrochemical windows but suffer from low ionic conductivity and poor interfacial compatibility, limiting their performance.
  • Existing challenges include inferior rate capability and inadequate cycling stability due to inherent material properties and interface issues.

Purpose of the Study:

  • To develop a novel amorphous solid electrolyte with enhanced ionic conductivity and interfacial compatibility for halides-based ASSLBs.
  • To investigate the effect of synergistic anion-cation modification on the local structure and ion transport properties of the solid electrolyte.
  • To demonstrate the improved electrochemical performance, including rate capability, cycling stability, and low-temperature operation, of ASSLBs utilizing the developed solid electrolyte.

Main Methods:

  • A synergistic anion-cation strategy was employed to modulate the local structure of halides-based solid electrolytes.
  • The amorphous solid electrolyte 1.6Li2O-TaCl5-0.3MgF2 (LTOC-M) was synthesized and characterized.
  • Electrochemical performance was evaluated using various cathode materials (LiNi0.8Co0.1Mn0.1O2, LiCoO2, Li-rich Li1.2Mn0.54Ni0.13Co0.13O2) and low-temperature conditions.

Main Results:

  • The amorphous solid electrolyte LTOC-M exhibited high ionic conductivity (11.15 mS cm−1) and favorable interfacial compatibility.
  • ASSLBs incorporating LTOC-M demonstrated superhigh rate capability and excellent long-term cycling stability with various cathode materials.
  • The developed ASSLBs showed remarkable performance at low temperatures, including operation at -75°C for over 400 hours.

Conclusions:

  • The synergistic anion-cation strategy effectively enhances the ionic conductivity and interfacial compatibility of halides-based solid electrolytes.
  • The developed amorphous solid electrolyte LTOC-M significantly improves the high-rate performance, long-term cycling stability, and low-temperature operation of ASSLBs.
  • This work provides a promising pathway for the practical application of halides-based ASSLBs in demanding conditions.