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Published on: June 30, 2018
Optical Torque Modulation of Cs2AgBiBr6 Perovskite-Coated Gold Nanospheres by Vector Bessel Beams
Ping Li1, Chen Yan1, Liangchen Lu1
1School of Physics, Xidian University, Xi'an 710071, China.
None:
Based on generalized Lorenz-Mie theory (GLMT) and the Maxwell stress tensor (MST) method, this study investigates the modulation mechanism of the axial optical torque Nz exerted on Cs2AgBiBr6 (CABB) perovskite-coated gold nanospheres under vector Bessel-beam illumination. The results show that the CABB shell reconstructs the torque-resonance channels of the coated particle by modifying both the dispersive dielectric environment around the gold core and the core-shell interfacial response. As the shell thickness increases, the dominant response undergoes a continuous redshift. The polarization state, half-cone angle α0, and order l of the incident vector Bessel beam serve as external optical-field degrees of freedom that regulate the incident angular-momentum channels, thereby enabling coordinated control over the torque peak magnitude, spectral line shape, and torque direction. Analyses of the near-field distributions, Poynting-vector distributions, and Mie-order decomposition reveal that the strong torque response arises from selective coupling between the intrinsic Mie channels of the core-shell particle and the vectorial structure of the incident light, rather than simply from local field-intensity enhancement. This study provides a theoretical basis for tunable Nz responses in perovskite-plasmonic hybrid nanostructures and for structured-light-driven rotational manipulation at the nanoscale.

