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Controlling Flow Speeds of Microtubule-Based 3D Active Fluids Using Temperature
Published on: November 26, 2019
Structure and memory control self-diffusion in active matter
Akinlade Akintunde1, Stewart A Mallory1,2
1Pennsylvania State University, Department of Chemistry, The , University Park, Pennsylvania 16802, USA.
None:
Despite extensive progress in characterizing the emergent behavior of active matter, the microscopic origins of self-diffusion in interacting active systems remain poorly understood. Here, we develop a framework that quantitatively links self-diffusion to collisional forces and their temporal correlations in active fluids. We show that transport is governed by two contributions: an equal-time suppression of motion arising from anisotropic collisional forces, and a memory correction associated with the temporal persistence of these forces. Together, these effects yield an exact expression for the self-diffusivity in terms of measurable force statistics and correlation times. We apply this framework to purely repulsive active Brownian particles and find that self-diffusion is always reduced as a function of packing fraction and activity. We identify the regimes in which equal-time force fluctuations and collisional memory dominate and how their relative contributions vary with activity and packing fraction. Our results establish a direct connection between microscopic force correlations and macroscopic transport, providing a general mechanical perspective for interpreting self-diffusion in active matter.
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