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Theoretical full-energy peak efficiency determination for LaBr3:Ce detectors
Ildefonso Riquelme Diaz1, Julio C Aguiar2
1Universidad Nacional de Asunción, Facultad de Ciencias Exactas y Naturales, (2160), Campus Universitario de San Lorenzo, Paraguay; Comisión Nacional de Energía Atómica, Campus Universitario de San Lorenzo 111401, Paraguay.
Abstract:
Lanthanum bromide scintillators doped with cerium, LaBr3:Ce, are widely used as room-temperature detectors for gamma-ray spectroscopy because of their good energy resolution, high detection efficiency, and fast timing response. Accurate modeling of their efficiency is therefore important for activity determination, efficiency calibration, and quantitative gamma-ray spectrometry. In this work, an analytical-semi-empirical formulation is presented for the full-energy peak efficiency of cylindrical LaBr3:Ce detectors. The efficiency is evaluated as the product of the total detection efficiency and the peak-to-total ratio. The total efficiency is calculated using analytical radiation-transport integrals for point, disk, and cylindrical volumetric sources positioned along the detector symmetry axis, building on classical total-efficiency formulations for cylindrical detectors. The peak-to-total ratio is described by a semi-empirical mean-chord-length formalism, with an energy-dependent parameter representing the average number of photon interactions inside the detector volume. The main contribution of the present approach is the combination of these analytical total-efficiency calculations with a peak-to-total formalism adapted to LaBr3:Ce detectors, together with an explicit self-attenuation correction for cylindrical volumetric sources. The resulting framework provides a computationally efficient and physically transparent tool for estimating full-energy peak efficiencies in well-defined axial geometries. The calculated efficiencies show good agreement with Monte Carlo simulations and experimental data reported in the literature.
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