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Phason-driven temperature-dependent transport in moiré graphene
Alex Boschi1, Alejandro Ramos-Alonso2, Vaidotas Mišeikis3
1Center for Nanotechnology Innovation, Istituto Italiano di Tecnologia, Piazza S. Silvestro 12, Pisa, 56127, Italy.
Abstract:
The electronic and vibrational properties of 2D materials are dramatically altered by the formation of a moiré superlattice. The lowest-energy phonon modes of the superlattice are two acoustic branches (calledphasons) that describe the sliding motion of one layer with respect to the other. Considering their low-energy dispersion and damping, these modes may act as a significant source of scattering for electrons in moiré materials. Here, we investigate temperature-dependent electrical transport in minimally twisted bilayer graphene, a moiré system developing multiple weakly-dispersive electronic bands and a reconstructed lattice structure. We measure a linear-in-temperature resistivity across the band manyfold aboveT∼ 10 K, preceded by a quadratic temperature dependence. While the linear-in-temperature resistivity is up to two orders of magnitude larger than in monolayer graphene, it is reduced (approximately by a factor of three) with respect to magic-angle twisted bilayer graphene. Moreover, it is modulated by the recursive band filling, with minima located close to the full filling of each band. Comparing our results with a semiclassical transport calculation, we show that the experimental trends are compatible with scattering processes mediated by longitudinal phasons, which dominate the resistivity over the contribution from conventional acoustic phonons of the monolayer. Our findings highlight the close relation between vibrational modes unique to moiré materials and carrier transport therein.