A table-top few-femtosecond broadband extreme-ultraviolet absorption spectrometer with cryogenic cooling
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Updated: Oct 31, 2026

High Resolution Phonon-assisted Quasi-resonance Fluorescence Spectroscopy
Published on: June 28, 2016
Sheng-Chih Lin1,2, Alfred Zong1,2,3,4, Emma Berger1,5
1Department of Chemistry, University of California at Berkeley, Berkeley, California 94720, USA.
Abstract:
We present a table-top cryogenic ultrafast broadband extreme-ultraviolet absorption spectroscopy beamline designed for temperature-dependent and time-resolved investigations of quantum materials. The instrument combines a broadband high-harmonic generation source spanning 22-73 eV with automated image registration and cryogenic sample control down to 20 K, enabling element-specific measurements under both equilibrium and nonequilibrium conditions. The beamline provides sub-50-meV energy resolution and a routine 10-fs instrument response function, while maintaining long-term stability suitable for extended, ultrasensitive measurements. Benchmark experiments on NiI2, a van der Waals multiferroic, reveal temperature-dependent spectral evolution across its magnetic phase transitions, demonstrating the ability to identify element-specific contributions to the ground state and its transient response in the femtosecond regime. This instrument introduces the opportunity to unravel the very first response of a solid-state material during light-matter interaction, paving the way for understanding the complex phase space of nonequilibrium dynamics and emergent states in strongly correlated systems where the few-femtosecond electronic response has eluded most other types of time-resolved techniques.
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