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Engineering Molecular Recognition with Bio-mimetic Polymers on Single Walled Carbon Nanotubes
Published on: January 10, 2017
Acoplamiento de un solo espín al movimiento de un nanotubo de carbono
Federico Fedele1, Federico Cerisola1,2, Lea Bresque3
1Dept. of Engineering Science, University of Oxford, Oxford, UK.
Abstract:
The ability to couple a solitary spin to high-frequency motion is a crucial advancement for a range of applications, including quantum sensing, intermediate and long-distance spin-spin coupling, and quantum information processing. Although proposed theoretically over a decade ago, experimental demonstrations have remained elusive. Here we report the observation of spin-mechanical coupling in a carbon nanotube device. We demonstrate this coupling in two configurations: off-resonant, with spin and mechanics excited by separate tones, and resonant, driven by a single tone. The coupling manifests as a shift and broadening of the electric dipole spin resonance (EDSR), respectively. Our theoretical model, which accounts for the tensor character of the coupling and mechanical non-linearity, reproduces the data with very good agreement. Our results demonstrate a previously unobserved spin-mechanical coupling, offering versatile tools for exploring macroscopic quantum phenomena, quantum thermodynamics, and quantum simulation.
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