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Updated: Jan 29, 2026

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末端のCo (III) -Oxo複合体によるCH活性化におけるpKa-駆動の非同期性に関する実験的証拠

McKenna K Goetz1, John S Anderson1

  • 1Department of Chemistry , University of Chicago , Chicago , Illinois 60637 , United States.

Journal of the American Chemical Society
|February 12, 2019
PubMed
まとめ

この研究では,C-H活性化におけるコバルト-オクソ複合体の反応性は,C-H結合強度ではなく,基板酸度 (pKa) によって導かれる. これは,移行金属オクソ複合体の新しい"非同期"の協調メカニズムを示唆しています.

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