在冬季北极平流层中检测到含有HNO3的大颗粒
D W Fahey1, R S Gao, K S Carslaw
1Aeronomy Laboratory, Climate Monitoring and Diagnostics Laboratory, National Oceanic and Atmospheric Administration, Boulder, CO 80305, USA. fahey@al.noaa.gov
概括
在北极平流层中观察到大量的酸颗粒,可能导致脱. 了解它们的形成是预测未来北极臭氧水平的关键.
科学领域:
- 大气化学 大气化学
- 石流层科学 石流层科学
- 北极研究研究北极研究
背景情况:
- 在1999/2000年北极冬季的平流层中观察到含有酸 (HNO3) 的大颗粒.
- 这些现场观测在几周内覆盖了广泛的海拔范围 (16-21公里) 和水平范围 (1800公里).
研究的目的:
- 调查北极平流层中大型酸颗粒的存在和特征.
- 评估这些粒子在较低层平流层引起脱的潜力.
- 了解这些粒子的形成机制,以便准确地预测臭氧丰度.
主要方法:
- 在1999/2000年北极冬季进行现场空中采样飞行.
- 对粒子大小 (10-20微米) 和组成 (酸) 的分析.
- 使用微物理模型模拟粒子生长和沉积.
主要成果:
- 对大型 (10-20微米) 酸三水合物颗粒的观察.
- 证明这些沉积颗粒具有显著的潜力,可以使下层平流层脱.
- 微物理模型成功模拟了粒子生长和沉积,但无法识别核化过程.
结论:
- 大型酸颗粒在北极脱过程中起着重要作用.
- 这些大颗粒的核化过程仍然未知.
- 准确的粒子形成建模对于理解北极臭氧损耗和未来预测至关重要.
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