在上层热层和下层平流层的离子核化过程中形成粒子
S-H Lee1, J M Reeves, J C Wilson
1Department of Engineering, University of Denver, Denver, CO 80208, USA. shanlee@du.edu
概括
在高层大气中,超细粒子度出乎意料地高. 离子诱导核化是这些大气粒子的关键来源,影响云形成和气候.
科学领域:
- 大气化学 大气化学
- 气溶科学 气溶科学
- 气候科学 气候科学
背景情况:
- 超细颗粒 (UFP) 在上层热层和下层平流层 (UTLS) 中普遍存在.
- 在UTLS中UFP的形成机制和来源仍然不完全理解.
- 之前的研究并没有充分考虑离子诱导核化作为该地区重要的UFP来源.
研究的目的:
- 研究在UTLS中超细颗粒的形成和生长.
- 确定离子诱导核化在UFP生产中的作用.
- 评估大气气溶中这种核化过程的全球意义.
主要方法:
- 使用了模拟离子诱导核化的数值模型.
- 用测量热力学数据进行受限模型模拟.
- 纳入大气中观察到的关键物种度.
主要成果:
- 模型模拟准确地复制了观察到的UFP数量度和尺寸分布.
- 发现离子诱导核化与UFP在UTLS的不同度的观测结果一致.
- 颗粒的形成和生长与足够的太阳辐射和较低的先前存在的气溶表面积有关.
结论:
- 离子诱导核化是UTLS新气溶颗粒的全球重要来源.
- 这些新形成的粒子在特定的大气条件下可以生长到可测量的尺寸.
- 这个过程对云的微物理和地球的辐射平衡有潜在的影响.
相关概念视频
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