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在现场催化剂改善了阿尔德化物以proline为媒介的α-amination

Hiroshi Iwamura1, Suju P Mathew, Donna G Blackmond

  • 1Department of Chemistry, Imperial College, London SW7 2AZ, UK.

Journal of the American Chemical Society
|September 24, 2004
PubMed
概括

林催化的α-氨基化反应表现出自我诱导的速率行为,并放大产品的反体过量. 这表明氨基酸催化可能解释生物同化性起源.

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Carbonyl compounds and primary amines undergo reductive amination first to produce imines, followed by secondary amines in the same reaction mixture, using selective reducing agents like sodium cyanoborohydride or sodium triacetoxyborohydride. Reductive amination produces different degrees of substitution of amines depending on the starting amine substrate.