概括
哥伦比亚河沉积物中含有的同位素比例表明了全球降落和当地来源. 来自汉福德核反应堆的-239对沉积物污染作出了重大贡献.
科学领域:
- 环境科学 环境科学
- 核化学 核化学 核化学
- 放射学评估 放射学评估
背景情况:
- 哥伦比亚河沉积物是环境污染物的沉池.
- 同位素来源于全球降落和当地核活动.
- 了解源对于环境修复和风险评估至关重要.
研究的目的:
- 为了调查哥伦比亚河沉积物中同位素的来源.
- 量化核反应堆历史运行对污染的贡献.
- 区分全球降落和河流环境中的的本地来源.
主要方法:
- 在沉积物样本中对同位素 (Pu-240,Pu-242,Pu-239) 进行质谱分析.
- 测量的同位素比率与已知的全球降落值的比较.
- 建模以估计反应堆衍生的的贡献.
主要成果:
- -240与-242的比率与全球降落模式一致.
- -240与-239的比率明显偏离了全球降落,这表明了另一个来源.
- 据估计,麦克纳里水库沉积物中约有20-25%的来自汉福德反应堆的运作.
结论:
- 哥伦比亚河沉积物显示出来自全球降落和汉福德工厂反应堆的混合签名.
- 来自汉福德的反应堆废水贡献了-239,它分解为-239,污染了沉积物.
- 当地核活动是下游沉积物中污染的重要,可量化的来源.
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