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减少的石墨烯氧化物作为固态电子介质在Z模式光催化水在可见光下分裂

Akihide Iwase1, Yun Hau Ng, Yoshimi Ishiguro

  • 1ARC Centre of Excellence for Functional Nanomaterials, School of Chemical Engineering, The University of New South Wales, Sydney, NSW 2052, Australia.

Journal of the American Chemical Society
|June 30, 2011
PubMed
概括

减少的石墨烯氧化物在Z模式光催化中起到有效的电子媒介作用,用于水分裂. 这种量身定制的材料使电子孔对的消耗增加了三倍,在可见光下增强和氧的生产.

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The Z-Scheme of Electron Transport in Photosynthesis01:34

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The light reactions of photosynthesis assume a linear flow of electrons from water to NADP+. During this process, light energy drives the splitting of water molecules to produce oxygen. However, oxidation of water molecules is a thermodynamically unfavorable reaction and requires a strong oxidizing agent. This is accomplished by the first product of light reactions: oxidized P680 (or P680+), the most powerful oxidizing agent known in biology. The oxidized P680 that acquires an electron from the...