通过胆固醇液晶的光子外进行放大光子向上转换
Ji-Hwan Kang, Shin-Hyun Kim1, Alberto Fernandez-Nieves
1Department of Chemical and Biomolecular Engineering, KAIST , Daejeon 305-701, South Korea.
Journal of the American Chemical Society
|April 14, 2017
概括
含有流体芯和胆固醇液晶外的微通过共振增强光子上转换 (TTA-UC). 这种设计使低值光子装置的光谱调整和放大发射成为可能.
科学领域:
- 光子学
- 材料科学
- 化学学
背景情况:
- 基于三倍-三倍-消灭的光子上转换 (TTA-UC) 是一个有前途的技术.
- 开发高效的TTA-UC平台需要先进的材料设计.
- 微流体技术提供了对微型结构制造的精确控制.
研究的目的:
- 创建具有流体TTA-UC核心和光子外的微囊.
- 在光子外中使用胆固醇液晶 (CLC).
- 调查这些微囊中的TTA-UC的光谱调和辐射放大.
主要方法:
- 作为模板的三重乳液的微流体制备
- 使用流体TTA-UC核心制造微囊.
- 将CLC与螺旋结构相结合,形成光子.
- 使用可聚合的半导体稳定CLC外.
主要成果:
- 该CLC光子外作为TTA-UC发射的共振腔.
- 在低功率激发下实现上转的光谱调整.
- 延迟光的全向放大发生在光子带间隙边缘.
- 微囊的设计显示了有效的TTA-UC增强.
结论:
- 微流体制备的微囊与CLC外对TTA-UC有效.
- 这种光子外可以实现共振,光谱调节和辐射放大.
- 这种方法为设计低值光子设备提供了巨大的潜力.
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