一个旋转轨道纠的量子液体在蜂格子上
K Kitagawa1, T Takayama2, Y Matsumoto2
1Department of Physics, University of Tokyo, Bunkyo-ku, Hongo 7-3-1, Tokyo 113-0033, Japan.
Nature
|February 16, 2018
概括
研究人员在H3LiIr2O6化合物中发现了一种量子自旋液体, 这一发现为探索外来准粒子提供了新的可能性.
科学领域:
- 凝聚物质物理学
- 材料科学
- 量子磁力学
背景情况:
- 蜂晶格中存在奇特的电子和自旋相,包括迪拉克费米子和量子自旋液体.
- 量子自旋液体是物质的无序状态,具有相互作用的自旋,缺乏对称性破坏.
- 之前的基塔耶夫量子自旋液体,如α-RuCl3,由于非基塔耶夫相互作用而表现出磁性排序.
研究的目的:
- 研究H3LiIr2O6作为量子自旋液体的潜力.
- 在强烈旋转轨道合的5d电子过渡金属氧化物中探索奇特的相和准粒子.
主要方法:
- 对H3LiIr2O6化合物的实验合成和表征.
- 低温测量包括核磁共振放松和特定热量.
- 分析磁性排序和低能费米离子激发.
主要成果:
- H3LiIr2O6表现出一个虚旋-1/2时的量子液态,没有磁顺序到0.05K.
- 尽管有强烈的相互作用 (~100 K),但没有观察到磁性秩序.
- 检测到低能费米离子激发的信号, 归因于旋转缺陷.
结论:
- H3LiIr2O6被确定为一个量子自旋液体.
- 这种材料为研究旋转轨道合系统中的奇异准粒子提供了一个有前途的平台.
相关概念视频
Quantum Numbers
52.4K
It is said that the energy of an electron in an atom is quantized; that is, it can be equal only to certain specific values and can jump from one energy level to another but not transition smoothly or stay between these levels.
52.4K
Atomic Orbitals
45.3K
An atomic orbital represents the three-dimensional regions in an atom where an electron has the highest probability to reside. The radial distribution function indicates the total probability of finding an electron within the thin shell at a distance r from the nucleus. The atomic orbitals have distinct shapes which are determined by l, the angular momentum quantum number. The orbitals are often drawn with a boundary surface, enclosing densest regions of the cloud.
45.3K
Lattice Centering and Coordination Number
12.6K
The structure of a crystalline solid, whether a metal or not, is best described by considering its simplest repeating unit, which is referred to as its unit cell. The unit cell consists of lattice points that represent the locations of atoms or ions. The entire structure then consists of this unit cell repeating in three dimensions. The three different types of unit cells present in the cubic lattice are illustrated in Figure 1.
Types of Unit Cells
Imagine taking a large number of identical...
Types of Unit Cells
Imagine taking a large number of identical...
12.6K
The Quantum-Mechanical Model of an Atom
59.8K
Shortly after de Broglie published his ideas that the electron in a hydrogen atom could be better thought of as being a circular standing wave instead of a particle moving in quantized circular orbits, Erwin Schrödinger extended de Broglie’s work by deriving what is now known as the Schrödinger equation. When Schrödinger applied his equation to hydrogen-like atoms, he was able to reproduce Bohr’s expression for the energy and, thus, the Rydberg formula governing hydrogen spectra.
59.8K
Electron Orbital Model
73.3K
Orbitals are the areas outside of the atomic nucleus where electrons are most likely to reside. They are characterized by different energy levels, shapes, and three-dimensional orientations. The location of electrons is described most generally by a shell or principal energy level, then by a subshell within each shell, and finally, by individual orbitals found within the subshells.
The first shell is closest to the nucleus, and it has only one subshell with a single spherical orbital called the...
The first shell is closest to the nucleus, and it has only one subshell with a single spherical orbital called the...
73.3K
Trends in Lattice Energy: Ion Size and Charge
26.8K
An ionic compound is stable because of the electrostatic attraction between its positive and negative ions. The lattice energy of a compound is a measure of the strength of this attraction. The lattice energy (ΔHlattice) of an ionic compound is defined as the energy required to separate one mole of the solid into its component gaseous ions. For the ionic solid sodium chloride, the lattice energy is the enthalpy change of the process:
26.8K


![Measuring the Spin-Lattice Relaxation Magnetic Field Dependence of Hyperpolarized [1-13C]pyruvate](/_next/image?url=https%3A%2F%2Fcloudfront.jove.com%2FCDNSource%2Fteasers%2F59399.jpg&w=3840&q=50)