在无电接触的异型二维PdSe2晶体中缺陷介导的相位转换
Akinola D Oyedele, Shize Yang, Tianli Feng1
1Department of Physics and Astronomy and Department of Electrical Engineering and Computer Science , Vanderbilt University , Nashville , Tennessee 37235 , United States.
Journal of the American Chemical Society
|May 16, 2019
概括
现在可以实现稳定的欧姆接触. 在二 (PdSe2) 中的相转换会产生金属相,形成无接触并提高晶体管的性能.
科学领域:
- 材料科学
- 凝聚物质物理学
- 纳米技术
背景情况:
- 实现稳定的欧姆接触对二维材料设备来说是一个关键的挑战.
- 目前的局限性阻碍了这些先进材料的性能和整合.
研究的目的:
- 展示一种在二维材料设备中创建无欧米接触的方法.
- 调查PdSe2中的相位转换以改善电特性.
主要方法:
- 使用等离子引发PdSe2的相变.
- 使用横截面扫描传输电子显微镜 (STEM).
- 使用理论计算来理解转换机制.
主要成果:
- 通过血诱导的空位成功形成了连续的金属Pd17Se15相.
- Pd17Se15/PdSe2的接口是原子利和化学结合.
- 接触者表现出低电阻 (∼0.75 kΩ μm) 和低斯科特基屏障高度 (∼3.3 meV).
- 与Ti/Au接触器相比,PdSe2晶体管的载体移动性增加了近20倍.
结论:
- 用等离子体诱导的相位转换为2D材料中稳定的欧米接触提供了可行的途径.
- 开发的方法显著提高了基于PdSe2的晶体管的性能.
- 这种方法为需要高效电气接触的二维材料的实际应用铺平了道路.
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