由于热驱动的旋转极化而引起的磁阻
Kouta Kondou1, Masanobu Shiga2, Shoya Sakamoto2
1Center for Emergent Matter Science (CEMS), RIKEN, Hirosawa, Wako Saitama 351-0198, Japan.
Journal of the American Chemical Society
|April 13, 2022
概括
这项研究揭示了奇拉分子中的一种新型磁阻,称为平面电流磁阻 (CIP-MR). 这种在室温下观察到的现象不需要电流通过分子,与以前的方法不同.
科学领域:
- 凝聚物质物理学
- 材料科学
- 分子电子
背景情况:
- 奇拉性诱导的电流垂直平面磁电阻 (CPP-MR) 与分子中电流诱导的旋转极化有关.
- 基拉尔诱导的自旋选择性 (CISS) 是基拉尔系统中控制自旋两极化的基本原理.
研究的目的:
- 在奇拉分子/铁磁金属双层中研究奇拉性诱导的平面电流磁阻 (CIP-MR).
- 探索CIP-MR背后的机制,特别是它与偏向电流的独立性.
- 了解热效应在分子旋转极化中的作用.
主要方法:
- 基质分子/铁磁金属双层的制造.
- 在室温下测量平面电流磁阻 (CIP-MR).
- 对CIP-MR的温度依赖性的分析.
主要成果:
- 在室温下观察到奇拉分子/铁磁金属双层中的新型CIP-MR.
- 证明CIP-MR不需要通过分子的偏向电流.
- CIP-MR的温度依赖表明热驱动的自发旋转偏振.
结论:
- 与金属表面接触的奇拉分子表现出有限的旋转极化.
- 热驱动的自发旋转极化是观察到的CIP-MR的关键机制.
- 这一发现符合并扩展了近期关于奇拉诱导旋转选择性的研究 (CISS).
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