在集群组装的Au6Te12Se8超导体中的超原子电荷密度波
Xu Chen1, Ge Fei2, Yanpeng Song1
1Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China.
Journal of the American Chemical Society
|October 27, 2022
概括
像Au6Te12Se8这样的超原子晶体显示了超原子电荷密度波 (S-CDW) 和超导电之间的压力诱导竞争. 外部压力显示出一个新的超导相与增强过渡温度.
科学领域:
- 凝聚物质物理学
- 材料科学
- 纳米技术
背景情况:
- 超原子晶体是由原子精确集群构成的等级材料.
- Au6Te12Se8是一种完全无机的超原子超导体,具有超原子电荷密度波 (S-CDW).
研究的目的:
- 研究超原子晶体对外压力的S-CDW和超导性的反应.
- 了解Au6Te12Se8中压力诱导的相变和导电性变化.
主要方法:
- 在现场同步X射线衍射.
- 理论上的计算.
- 在不同压力下进行运输测量.
主要成果:
- 对于应对外部压力而言,S-CDW具有低压值 (0.1 GPa).
- 第二个超导相在7.3GPa以上出现,将过渡温度 (Tc) 提高到8.5K.
- 压力诱导超原子滑动和费米表面拓过渡,导致导电度的维度交叉.
结论:
- Au6Te12Se8显示了S-CDW和超导之间的独特的压力依赖相互作用.
- 观察到的回流超导与导电性和费米表面拓的维度交叉有关.
- 超原子晶体为探索压力下的量子现象提供了一个新平台.
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