数据融合和多变量分析用于食品真实性分析
Yunhe Hong1, Nicholas Birse1, Brian Quinn1
1National Measurement Laboratory: Centre of Excellence in Agriculture and Food Integrity, Institute for Global Food Security, School of Biological Sciences, Queen's University Belfast, Belfast, United Kingdom.
Nature communications
|June 8, 2023
概括
通过将两种质谱法与数据分析相结合,可以准确识别鱼的来源和生产. 这种双平台方法实现了100%的准确性,超越了食品真实性的单一方法的限制.
科学领域:
- 分析化学 分析化学
- 食品科学 食品科学 食品科学
- 化学测量 化学测量 化学测量
背景情况:
- 准确确定食品原产地和生产方法对于消费者信任和监管合规至关重要.
- 单一的分析平台往往难以为像鱼这样的复杂食物矩阵提供全面的数据.
- 开发可靠的食品来源方法对于打击欺诈和确保质量至关重要.
研究的目的:
- 开发和验证一种新的数据融合方法,用于分类鱼的来源和生产方法.
- 评估结合快速蒸发电离质谱 (REIMS) 和感应合等离子体质谱 (ICP-MS) 数据的有效性.
- 为了识别可靠的化学标记,表明鱼的来源.
主要方法:
- 采用了中级数据融合策略,整合了REIMS和ICP-MS的数据.
- 多变量分析技术应用于合并的数据集.
- 分析了来自五个地区和两种生产类型的522个鱼样本的研究队列.
主要成果:
- 双平台数据融合实现了对鱼来源和生产的100%交叉验证分类准确性.
- 所有17个测试样本都被正确地根据原产地识别出来,这是单平台方法无法实现的壮举.
- 18种脂质标记物和9种元素标记物被确定为鱼来源的强有力的指标.
结论:
- 综合数据融合和多变量分析策略显著提高了识别鱼地理来源和生产方法的准确性.
- 这种创新方法显示出在更广泛的食品真实性和可追溯性挑战中应用的巨大潜力.
- 双平台质谱为复杂的食品认证问题提供了强大的解决方案.
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