在二维铁磁半导体异构结构中的反铁磁-铁磁切换的超快激光控制
Zhaobo Zhou1, Zhenfa Zheng2, Junjie He3
1Bremen Center for Computational Materials Science, University of Bremen, Bremen 28359, Germany.
Nano letters
|June 12, 2023
概括
超快激光脉冲控制CrCl3/CrBr3异构中的磁化切换. 这项研究揭示了将反铁磁转换为铁磁顺序的新机制,为先进的光旋电子设备铺平了道路.
科学领域:
- 凝聚物质物理学 凝聚物质物理学
- 材料科学 材料科学 材料科学
- 量子光学是一种量子光学.
背景情况:
- 超快的磁化控制对于下一代信息技术至关重要.
- 探索2D磁性异构结构中的激光诱导动力学是开发新型自旋电子设备的关键.
研究的目的:
- 在CrCl3/CrBr3异构结构中研究激光诱导的自旋电子激发和放松.
- 了解反平行 (AP) 和平行 (P) 系统中磁化切换背后的机制.
- 探索超快激光控制在二维 (2D) 光旋电子器件中的潜力.
主要方法:
- 激光诱导的自旋电子激发和放松动态的理论探索.
- 在AP和P两种配置中分析CrCl3/CrBr3异构.
- 微观机制调查涉及电荷转移和旋转转动力学.
主要成果:
- 在AP和P系统中观察到超快的去磁化,由于相当的层间激发,整体磁性秩序被保留.
- 关键的是,AP系统显示了从反铁磁 (AFM) 切换到铁磁 (FiM) 后激光脉冲的顺序.
- 确定了不对称的层间电荷转移和旋转翻转作为AFM切换到FiM的主导机制.
结论:
- 激光诱导的现象可以有效地控制2D异构结构中的磁化切换.
- 发现的机制为超快的磁场光学控制提供了一个新的途径.
- 这项研究为设计用于信息处理的先进二维光旋电子设备开辟了道路.
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