尼克莱酸盐和一些基于铁的超导体中的内在连贯度长度异质性
1M. N. Miheev Institute of Metal Physics, Ural Branch, Russian Academy of Sciences, 18, S. Kovalevskoy St., 620108 Ekaterinburg, Russia.
Materials (Basel, Switzerland)
|June 28, 2023
概括
2019年发现的酸超导体,在薄膜中表现出独特的超导特性,但不是批量. 一个新的3D模型解释了它们的关键磁场行为,表明它们不是纯粹的2D超导体.
科学领域:
- 超导电性 超导电性 超导电性
- 材料科学 材料科学 材料科学
- 凝聚物质物理学 凝聚物质物理学
背景情况:
- 尼基酸超导体 (R1-xAxNiO2) 在2019年被发现,仅在薄膜中表现出超导性 (Tc高达18K),这种现象在散装材料中没有观察到.
- 尼基酸盐的温度依赖的上临界场 (Bc2(T)) 通常使用2D模型进行分析,但推断的参数通常与物理薄膜尺寸相矛盾.
- 现有的二维超导模型假定薄膜厚度和连贯度长度 (ξab(0), ξc(0) 之间存在特定的关系,这些关系在酸薄膜中被发现被侵犯.
研究的目的:
- 为了解决分析尼基酸超导体关键场数据中的差异.
- 提出和验证一种新的分析三维 (3D) 模型,用于在尼基酸盐中适配在平面内和平面外的Bc2{\displaystyle Bc2}{\displaystyle Bc2}{\displaystyle Bc2}{\displaystyle Bc2}{\displaystyle Bc2}{\displaystyle Bc2}{\displaystyle Bc2}{\displaystyle Bc2}{\displaystyle Bc2}{\displaystyle Bc2}{\displaystyle T}).
- 为了研究在薄膜尼基酸盐中观察到的超导行为背后的原因.
主要方法:
- 对R1-xAxNiO2膜中温度依赖的上临界场 (Bc2(T)) 的报告实验数据的分析.
- 开发一个分析的3D模型,结合温度依赖的连贯长度异构的启发式表达式: γξ(T) = γξ(0) [1 - (T/Tc) a],其中"a"是一个合适的参数.
- 应用3D模型,使Bc2{\displaystyle Bc2{\displaystyle T}的总数据适合不同的维度.
主要成果:
- 实验数据分析显示,对于R1-xAxNiO2膜,二维超导模型的条件没有得到满足.
- 拟议的3D模型成功地为尼基酸盐中的平面内和平面外Bc2(T) 数据提供了全局匹配.
- 连贯长度异构的启发式表达式证明了更广泛的适用性,也适用于散装pnictide和 chalcogenide超导体的数据.
结论:
- 呈现超导性的酸薄膜不像纯二维超导体那样表现,这与基于配合模型的初步假设相反.
- 开发的3D分析模型更准确地描述了酸盐的超导特性.
- 拟议的模型及其对连贯长度异构的基本表达式显示了在理解各种超导材料方面更广泛应用的潜力.
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