在Bi2Te3的表面运输的定位和方向性有序的3D纳米网络
Alejandra Ruiz-Clavijo1, Nicolás Pérez2, Olga Caballero-Calero1
1Instituto de Micro y Nanotecnología, IMN-CNM, CSIC (CEI UAM+CSIC) Isaac Newton 8, E-28760, Tres Cantos, Madrid, Spain.
ACS nano
|July 6, 2023
概括
3D-Bi2Te3纳米线纳米网络的电阻显示安德森定位低于50K. 弱反定位表示沿垂直纳米线方向运输,增强Seebeck系数.
科学领域:
- 凝聚物质物理学 凝聚物质物理学
- 材料科学 材料科学 材料科学
- 纳米技术 纳米技术
背景情况:
- 了解纳米结构材料中的电子运输对于热电应用至关重要.
- 石棉化物 (Bi2Te3) 纳米线是有前途的热电材料.
- 维度和形态对电子定位的影响是一个活跃的研究领域.
研究的目的:
- 在低温下研究3D-Bi2Te3纳米线纳米网络的电阻和磁阻.
- 了解底层的电子传输机制和局部化效应.
- 为了将运输特性与热电性能相关联.
主要方法:
- 低温电阻测量. 低温电阻测量.
- 取决于角度的磁电阻测量.
- 使用安德森模型进行本地化和Hikami-Larkin-Nagaoka模型进行分析.
主要成果:
- 阻力增加到50K以下,这与安德森在平行通道中的定位一致.
- 观察到微弱的反局部化,表明沿垂直纳米线轴进行运输.
- 确定一致度长度:跨纳米线的~700nm,沿单个纳米线的~100nm.
- 定位效应与增强的西贝克系数相关.
结论:
- 在3D-Bi2Te3纳米线纳米网络中,电子运输受局部化现象的控制.
- 纳米网络结构促进了独特的传输路径,影响了连贯长度.
- 观察到的本地化效应是纳米网络增强的Seebeck系数的一个关键因素.
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