作为长期地质化学档案的历史建筑环境:在城市"污染钟"上告诉时间
Katrin Wilhelm1, Jack Longman2,3, Christopher D Standish4
1Oxford Resilient Buildings and Landscapes Laboratory (OxRBL), School of Geography and the Environment, University of Oxford, South Parks Road, Oxford, OX1 3QY, U.K.
Environmental science & technology
|July 12, 2023
概括
历史建筑充当地化学档案,揭示城市空气污染的变化. 对黑皮的同位素分析表明,燃煤占主导地位的早期污染,其他来源,如含汽油,后来出现.
科学领域:
- 环境科学 环境科学
- 地质化学 地质化学
- 考古测量考古测量方法
背景情况:
- 城市环境缺乏可靠的档案来重建历史污染.
- 历史悠久的建筑物在几个世纪以来积累了大气污染物.
研究的目的:
- 开发一种使用历史建筑作为地化学档案的新方法.
- 使用同位素分析重建过去的城市空气污染标志.
主要方法:
- 高分辨率激光除质谱仪用于同位素分析 (206Pb/207Pb和208Pb/206Pb).
- 从350年前的历史结构中分析黑色地层状图.
- 质量平衡分析以确定源贡献.
主要成果:
- 黑色的皮层显示了随着时间的推移,同位素比率的变化,这表明了来源的变化.
- 自1669年以来形成的层有>90%的煤炭燃烧的.
- 现代污染源,包括含汽油,从1875年开始占主导地位 (高达60%).
结论:
- 历史建筑环境是有价值的,用于空气污染研究的本地化地化学档案.
- 这种方法通过提供城市特定的污染数据来补充全球档案.
- 了解历史污染动态可以提高对人类对城市环境影响的了解.
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