在剪切加厚悬浮液中,粘度和扩散度之间的缩放关系
Abhinendra Singh1, Kuniyasu Saitoh2
1Department of Macromolecular Science and Engineering, Case Western Reserve University, Cleveland, Ohio 44106, USA. abhinendra.singh@case.edu.
Soft matter
|August 21, 2023
概括
颗粒粘度和扩散随着剪切应力增加,这是由于滑到摩擦过渡. 一个通用关系通过粒子集群大小将粘度和扩散度连接到不同的流程中.
科学领域:
- 物理 物理学 物理
- 材料科学 材料科学 材料科学
- 化学工程是化学工程的重要组成部分.
背景情况:
- 密集悬浮在变形下表现出复杂的行为.
- 这些行为与滑和摩擦状态之间的过渡有关.
研究的目的:
- 调查摩擦非布罗恩球体的流动行为和剪切引起的扩散.
- 建立粘度和扩散度之间的关系.
主要方法:
- 2D简单剪流的数值模拟.
- 对摩擦非布罗恩球体的分析.
主要成果:
- 粘度 (η) 和扩散度 (D/τ) 随着特有的剪切应力而增加,这表明滑向摩擦过渡.
- 建议在粘度和扩散性之间建立一对一的关系,由粒子集群的长度尺度 (ξ) 支配.
- 这种关系显示了D/τ ∼ η在无摩擦状态到D/τ ∼ η^(1/3) 在摩擦状态的交叉.
结论:
- 这项研究揭示了密集的摩擦悬浮物中粘度和扩散率之间的普遍关系.
- 这种关系是由粒子集群大小控制的,并且独立于粒子间摩擦和系统大小.
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